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Decomposition analysis of energy-related carbon dioxide emissions in the iron and steel industry in China

Wenqiang SUN, Jiuju CAI, Hai YU, Lei DAI

《环境科学与工程前沿（英文）》 2012年第6卷第2期页码 265-270 doi: 10.1007/s11783-011-0284-8

摘要： This work aims to identify the main factors influencing the energy-related carbon dioxide (CO ) emissions from the iron and steel industry in China during the period of 1995–2007. The logarithmic mean divisia index (LMDI) technique was applied with period-wise analysis and time-series analysis. Changes in energy-related CO emissions were decomposed into four factors: emission factor effect, energy structure effect, energy consumption effect, and the steel production effect. The results show that steel production is the major factor responsible for the rise in CO emissions during the sampling period; on the other hand the energy consumption is the largest contributor to the decrease in CO emissions. To a lesser extent, the emission factor and energy structure effects have both negative and positive contributions to CO emissions, respectively. Policy implications are provided regarding the reduction of CO emissions from the iron and steel industry in China, such as controlling the overgrowth of steel production, improving energy-saving technologies, and introducing low-carbon energy sources into the iron and steel industry.

关键词： carbon dioxide (CO₂) emissions decomposition analysis logarithmic mean divisia index (LMDI) technique time-series analysis

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Scale up of reactors for carbon dioxide reduction

《化学科学与工程前沿（英文）》 2023年第17卷第1期页码 116-122 doi: 10.1007/s11705-022-2178-7

摘要： In recent times there has been a great deal of interest in the conversion of carbon dioxide into more useful chemical compounds. On the other hand, the translation of these developments in electrochemical reduction of carbon dioxide from the laboratory bench to practical scale remains an underexplored topic. Here we examine some of the major challenges, demonstrating some promising strategies towards such scale-up, including increased electrode area and stacking of electrode pairs in different configurations. We observed that increasing the electrode area from 1 to 10 cm² led to only a 4% drop in current density, with similarly small penalties realised when stacking sub-cells together.

关键词： CO₂ reduction electrochemical cell electrosynthesis upscaling

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Methanation of carbon dioxide: an overview

Wei WANG, Jinlong GONG

《化学科学与工程前沿（英文）》 2011年第5卷第1期页码 2-10 doi: 10.1007/s11705-010-0528-3

摘要： Although being very challenging, utilization of carbon dioxide (CO ) originating from production processes and flue gases of CO -intensive sectors has a great environmental and industrial potential due to improving the resource efficiency of industry as well as by contributing to the reduction of CO emissions. As a renewable and environmentally friendly source of carbon, catalytic approaches for CO fixation in the synthesis of chemicals offer the way to mitigate the increasing CO buildup. Among the catalytic reactions, methanation of CO is a particularly promising technique for producing energy carrier or chemical. This article focuses on recent developments in catalytic materials, novel reactors, and reaction mechanism for methanation of CO .

关键词： CO₂ methanation hydrogenation catalysis methane environmental science

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Enhancing the aromatic selectivity of cyclohexane aromatization by CO2sub> coupling

《化学科学与工程前沿（英文）》 2023年第17卷第11期页码 1801-1808 doi: 10.1007/s11705-023-2325-9

摘要： Improving the aromatic selectivity in the alkane aromatization process is of great importance for its practical utilization but challenge to make because the high H/C ratio of alkanes would lead to a serious hydrogen transfer process and a large amount of light alkanes. Herein, CO₂ is introduced into the cyclohexane conversion process on the HZSM-5 zeolite, which can improve the aromatic selectivity. By optimizing the reaction conditions, an improved aromatic (benzene, toluene, xylene, and C₉₊) selectivity of 48.2% can be obtained at the conditions of 2.7 MPa (CO₂), 450 °C, and 1.7 h⁻¹, which is better than that without CO₂ (aromatic selectivity = 43.2%). In situ transmission Fourier transform infrared spectroscopy spectra illustrate that many oxygenated chemical intermediates (e.g., carboxylic acid, anhydride, unsaturated aldehydes/ketones or ketene) would be formed during the cyclohexane conversion process in the presence of CO₂. ¹³C isotope labeling experimental results demonstrate that CO₂ can enter into the aromatics through the formation of oxygenated chemical intermediates and thereby improve the aromatic selectivity. This study may open a green, economic, and promising way to improve the aromatic selectivity for alkane aromatization process.

关键词： aromatics carbon dioxide aromatization coupling reaction ZSM-5 zeolite

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A state-of-the-art review of solar passive building system for heating or cooling purpose

Arun Kumar NANDA,C K PANIGRAHI

《能源前沿（英文）》 2016年第10卷第3期页码 347-354 doi: 10.1007/s11708-016-0403-0

摘要： The major portion of energy in a building is consumed by heating, ventilating, and air-conditioning (HVAC). The traditional heating and cooling systems contribute greatly to the emission of greenhouse gases, especially carbon dioxide. Four different ways, i.e., Trombe wall, solar chimney, unglazed transpired solar façade, and solar roof, are adopted for solar heating. Similarly, two major ways, i.e., evaporative cooling and building integrated evaporative cooling are adopted for cooling of the building. Therefore, an attempt has been made in this paper to compile the developments of solar heating and cooling technologies in a building.

关键词： HVAC heating cooling solar heating carbon dioxide (CO₂) emissions

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太阳能技术对我国未来减排CO2sub> 的贡献

赵玉文

《中国工程科学》 2003年第5卷第4期页码 38-40

摘要：

在“我国后续能源发展战略研究”基础上对太阳能技术在我国未来减排CO2sub>中的作用进行了估计，结果表明，在2010年后太阳能技术对CO2sub

关键词：太阳能，CO2减排

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Frontier science and challenges on offshore carbon storage

《环境科学与工程前沿（英文）》 2023年第17卷第7期 doi: 10.1007/s11783-023-1680-6

摘要：

● The main direct seal up carbon options and challenges are reviewed.

关键词： Offshore carbon storage Direct CO₂ injection CO₂-CH₄ replacement CO₂-EOR CCS hubs CO₂ transport

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粤港澳大湾区CO2sub>排放趋势、驱动因素及减排路径 Article

周雅, 李柯君, 梁笙, 曾雪兰, 蔡宴朋, 孟靖, 单钰理, 关大博, 杨志峰

《工程（英文）》 2023年第23卷第4期页码 138-148 doi: 10.1016/j.eng.2022.03.017

摘要：

粤港澳大湾区是我国为建设世界级城市群提出的国家战略，其CO2sub>排放趋势、社会经济驱动因素和减排路径对区域经济高质量发展具有重要意义。本研究编制了2000—2019 年粤港澳大湾区CO2sub>排放清单，采用对数平均迪氏指数法探究CO2sub>排放的关键驱动力。结果表明，粤港澳大湾区CO2sub>排放在2017 年后明显放缓，已经与国内生产总值（GDP）增长脱钩。经济增长和能源强度分别是驱动和抑制粤港澳大湾区CO2sub>排放增加的主要因素。能源生产和重工业对粤港澳大湾区CO2sub>排放增长的推动作用降低，服务业正成为主要驱动力。深圳和香港的产业升级以及深圳、广州和佛山的技术进步抑制了粤港澳大湾区CO2sub>排放增长。粤港澳大湾区各城市异质性增加了减排指标分配难度和制定区域碳中和路线图的复杂性。

关键词：粤港澳大湾区 CO2sub>排放驱动因素低碳发展碳中和

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以净零排放为目标的封存驱动型CO2sub>提高采收率方法 Article

刘月亮, 芮振华

《工程（英文）》 2022年第18卷第11期页码 79-87 doi: 10.1016/j.eng.2022.02.010

摘要：可通过驱油过程将CO2sub>封存在油藏地质体中，因此，CO2sub>驱油与封存被视为降低CO2sub>排放的重要手段之一。本研究提出了一种新型的CO2sub>提高采收率（EOR）方法，即封存驱动型CO2sub>提高采收率，其主要目标是通过在油藏中封存尽可能多的CO2sub>来实现CO结果表明，DME可提高CO2sub>在原油中的溶解度，有利于CO2sub>的溶解封存；可抑制因CO2sub>的抽提作用造成的原油轻质组分“逃逸&rdquo封存驱动型CO2sub> EOR方法在提高波及效率方面优于传统的CO2sub> EOR，尤其是在采油后期更为明显；同时，封存驱动型CO2sub> EOR比传统的此外，通过封存驱动型CO2sub> EOR封存的CO2sub>量远超采出原油燃烧产生的碳排放总量。

关键词： CO2sub> EOR CO2sub>净排放量二甲醚封存驱动型CO2sub> EOR CO2sub>封存

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Reducing CO emissions from the rebalancing operation of the bike-sharing system in Beijing

《工程管理前沿（英文）》 2023年第10卷第2期页码 262-284 doi: 10.1007/s42524-021-0168-y

摘要： With the development of the bike-sharing system (BSS) and the introduction of green and low carbon development, the environmental impacts of BSS had received increasing attention in recent years. However, the emissions from the rebalancing of BSS, where fossil-fueled vehicles are commonly used, are usually neglected, which goes against the idea of green travel in a sharing economy. Previous studies on the bike-sharing rebalancing problem (BRP), which is considered NP-hard, have mainly focused on algorithm innovation instead of improving the solution model, thereby hindering the application of many existing models in large-scale BRP. This study then proposes a method for optimizing the CO₂ emissions from BRP and takes the BSS of Beijing as a demonstration. We initially analyze the spatial and temporal characteristics of BSS, especially the flow between districts, and find that each district can be independently rebalanced. Afterward, we develop a rebalancing optimization model based on a partitioning strategy to avoid deciding the number of bikes being loaded or unloaded at each parking node. We then employ the tabu search algorithm to solve the model. Results show that (i) due to over launch and lack of planning in rebalancing, the BSS in Beijing shows great potential for optimization, such as by reducing the number of vehicle routes, CO₂ emissions, and unmet demands; (ii) the CO₂ emissions of BSS in Beijing can be reduced by 57.5% by forming balanced parking nodes at the end of the day and decreasing the repetition of vehicle routes and the loads of vehicles; and (iii) the launch amounts of bikes in specific districts, such as Shijingshan and Mentougou, should be increased.

关键词： bike-sharing CO₂ emissions environmental benefit partitioning strategy rebalancing problem

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Peak CO

Sheng ZHOU, Maosheng DUAN, Zhiyi YUAN, Xunmin OU

《能源前沿（英文）》 2020年第14卷第4期页码 740-758 doi: 10.1007/s11708-018-0558-y

摘要： This paper studies the pathways of peaking CO emissions of Dezhou city in China, by employing a bottom-up sector analysis model and considering future economic growth, the adjustment of the industrial structure, and the trend of energy intensity. Two scenarios (a business-as-usual (BAU) scenario and a CO mitigation scenario (CMS)) are set up. The results show that in the BAU scenario, the final energy consumption will peak at 25.93 million tons of coal equivalent (Mtce) (16% growth versus 2014) in 2030. In the CMS scenario, the final energy will peak in 2020 at 23.47 Mtce (9% lower versus peak in the BAU scenario). The total primary energy consumption will increase by 12% (BAU scenario) and decrease by 3% (CMS scenario) in 2030, respectively, compared to that in 2014. In the BAU scenario, CO emission will peak in 2025 at 70 million tons of carbon dioxide (MtCO ), and subsequently decrease gradually in 2030. In the CMS scenario, the peak has occurred in 2014, and 60 MtCO will be emitted in 2030. Active policies including restructuring the economy, improving energy efficiency, capping coal consumption, and using more low-carbon /carbon free fuel are recommended in Dezhou city peaked CO emission as early as possible.

关键词： carbon dioxide emission energy consumption peak CO₂ emission low-carbon transition Dezhou city China

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Revealing the GHG reduction potential of emerging biomass-based CO utilization with an iron cycle system

《环境科学与工程前沿（英文）》 2023年第17卷第10期 doi: 10.1007/s11783-023-1727-8

摘要：

● Greenhouse gas mitigation by biomass-based CO₂ utilization with a Fe cycle system.

关键词： Carbon dioxide utilization Hydrothermal reactions Biomass-based CO₂ reduction Simulation Ex-ante LCA

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Greenhouse gas emissions during co-composting of cattle feedlot manure with construction and demolition

Xiying Hao, Francis J. Larney

《环境科学与工程前沿（英文）》 2017年第11卷第3期 doi: 10.1007/s11783-017-0955-1

摘要： Manure management strategies should reflect current animal feeding practices and encourage recycling of organic waste to help protect our environment. This research investigated greenhouse gas (GHG) emissions during cattle manure stockpiling or composting with and without construction and demolition (C&D) waste. Manure was collected from cattle fed a typical finishing diet (CK manure) and from cattle on diets which included 30% dried distillers grains with solubles (DG manure). The CK and DG manures were co-composted with (4:1) C&D waste (treatments: CK_CD DG_CD), composted alone (treatments: CK and DG) in 13 m bins or stockpiled without C&D waste (treatments: CK_ST and DG_ST) for 99 days. Manure type (CK vs. DG manure) had no effect on GHG emissions over the 99 day manure composting or stockpiling. Composting with C&D waste produced similar CO emissions, about double that from manure stockpiling (7.0 kgC·m ). In contrast, CH emissions were reduced by the inclusion of C&D waste (64 gC·m with C&D vs. 244 gC·m without C&D) while the manure stockpile emitted the greatest amount of CH (464 gC·m ). Additionally, only 0.48% of C was emitted in CH form with C&D waste, compared to 1.68% when composting without C&D waste and 7.00% when cattle manure was stockpiled. The N O emissions (12.4 to 18.0 gN·m ) were similar across all treatments. The lower CH emissions with C&D waste are beneficial in reducing overall GHG emissions from manure composting, while reducing the amount of material entering landfills.

关键词： Livestock manure greenhouse gas flux straw bale compost bin N₂O CH₄ CO₂

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Activated carbons and amine-modified materials for carbon dioxide capture –– a review

Zhenhe CHEN, Shubo DENG, Haoran WEI, Bin WANG, Jun HUANG, Gang YU

《环境科学与工程前沿（英文）》 2013年第7卷第3期页码 326-340 doi: 10.1007/s11783-013-0510-7

摘要： Rapidly increasing concentration of CO in the atmosphere has drawn more and more attention in recent years, and adsorption has been considered as an effective technology for CO capture from the anthropogenic sources. In this paper, the attractive adsorbents including activated carbons and amine-modified materials were mainly reviewed and discussed with particular attention on progress in the adsorbent preparation and CO adsorption capacity. Carbon materials can be prepared from different precursors including fossil fuels, biomass and resins using the carbonization-activation or only activation process, and activated carbons prepared by KOH activation with high CO adsorbed amount were reviewed in the preparation, adsorption capacity as well as the relationship between the pore characteristics and CO adsorption. For the amine-modified materials, the physical impregnation and chemical graft of polyethylenimine (PEI) on the different porous materials were introduced in terms of preparation method and adsorption performance as well as their advantages and disadvantages for CO adsorption. In the last section, the issues and prospect of solid adsorbents for CO adsorption were summarized, and it is expected that this review will be helpful for the fundamental studies and industrial applications of activated carbons and amine-modified adsorbents for CO capture.

关键词： adsorption capacity CO₂ capture activated carbon amine-impregnated adsorbents

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Decomposition analysis applied to energy and emissions: A literature review

《工程管理前沿（英文）》页码 625-639 doi: 10.1007/s42524-023-0270-4

摘要： Decomposition analysis has been widely used to assess the determinants of energy and CO₂ emissions in academic research and policy studies. Both the methodology and application of decomposition analysis have been largely improved in the past decades. After more than 50 years’ developments, decomposition studies have become increasingly sophisticated and diversified, and tend to converge internally and integrate with other analytical approaches externally. A good understanding of the literature and state of the art is critical to identify knowledge gaps and formulate future research agenda. To this end, this study presents a literature survey for decomposition analysis applied to energy and emission issues, with a focus on the period of 2016–2021. A review for three individual decomposition techniques is first conducted, followed by a synthesis of emerging trends and features for the decomposition analysis literature as a whole. The findings are expected to direct future research in decomposition analysis.

关键词： index decomposition analysis structural decomposition analysis production decomposition analysis energy CO₂ emissions